Burgess Meredith

Dr. Diabolo (Framing Story)

Jack Palance

Ronald Wyatt (segment 4 "The Man Who Collected Poe")

Beverly Adams

Carla Hayes (segment 2 "Terror Over Hollywood")

Peter Cushing

Lancelot Canning (segment 4 "The Man Who Collected Poe")

Maurice Denham

Uncle Roger (segment 1 "Enoch")

Barbara Ewing

Dorothy Endicott (segment 3 "Mr. Steinway")

Michael Bryant

Colin Williams (segment 1 "Enoch")

John Standing

Leo Winston (segment 3 "Mr. Steinway")